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Decoration engineering induced MoS(2)QDs/BiOBr heterostructures for significantly enhancing visible light photocatalytic capability for the organic dyes and antibiotics removal

  ( SCI-EXPANDED收录)  

文献类型:期刊文献

英文题名:

Decoration engineering induced MoS(2)QDs/BiOBr heterostructures for significantly enhancing visible light photocatalytic capability for the organic dyes and antibiotics removal

作者:Zhang, Mingliang[1,2];Duo, Fangfang[2];Lan, Jihong[2];Li, Lixiang[1];Zhou, Jianwei[2];Chu, Liangliang[2];Wang, Chubei[2]

第一作者:Zhang, Mingliang;张明亮

通讯作者:Li, LX[1];Duo, FF[2]

机构:[1]Univ Sci & Technol Liaoning, Sch Chem Engn, 185 Qianshanzhong Rd, Anshan 114051, Liaoning, Peoples R China;[2]Xinxiang Univ, Henan Photoelectrocatalyt Mat & Micronano Applica, Xinxiang 453003, Henan, Peoples R China

第一机构:Univ Sci & Technol Liaoning, Sch Chem Engn, 185 Qianshanzhong Rd, Anshan 114051, Liaoning, Peoples R China

通讯机构:[1]corresponding author), Univ Sci & Technol Liaoning, Sch Chem Engn, 185 Qianshanzhong Rd, Anshan 114051, Liaoning, Peoples R China;[2]corresponding author), Xinxiang Univ, Henan Photoelectrocatalyt Mat & Micronano Applica, Xinxiang 453003, Henan, Peoples R China.|[11071]新乡学院;

年份:2022

卷号:583

外文期刊名:APPLIED SURFACE SCIENCE

收录:;WOS:【SCI-EXPANDED(收录号:WOS:000773627500005)】;

基金:Acknowledgements The authors gratefully acknowledge the financial support provided by the Natural Science Found of China (No. 51872131, 51102126 and 51672118) and Key Scientific Research Projects of Institutions of Higher Learning in Henan Province (22B150014) .

语种:英文

外文关键词:MoS2 quantum dots; Heterojunction; Photocatalytic; Rhodamine B; Ciprofloxacin

摘要:A novel MoS2 quantum dots decorated BiOBr heterostructure photocatalyst has been successfully fabricated by a facile hydrolysis approach. The MoS(2)QDs are prepared through an ultrasound-exfoliation method by MoS2 nanosheet. The structure, morphology, elemental composition and optical absorption properties of materials have been detailedly investigated by X-ray powder diffraction (XRD), FT-IR spectrum, Raman spectrum, scanning electron microscopy, transmission electron microscopy (TEM), high-resolution TEM (HRTEM), energy dispersive spectrometer (EDS), X-ray photoelectron spectroscopy (XPS), UV-vis diffuse reflectance spectroscopy (DRS) and photoluminescence spectra (PL), respectively. It can be observed that MoS(2)QDs with a diameter of about 5 nm are uniformly and firmly dispersed on the surface of the BiOBr. The MoS(2)QDs/BiOBr heterostructures show excellent photocatalytic activity both towards rhodamine B dyes and ciprofloxacin under visible light irradiation. It can be attributed to the synergistic effect of MoS(2)QDs/BiOBr heterostructures between MoS(2)QDs and BiOBr, which can promote the separation of photo-induced carriers and absorption of visible light. A heterojunction model based on the charges transfer mechanism has been proposed. Furthermore, the scavenger experiments and repeated experiments are conducted. The superior photocatalytic activity and excellent stability of MoS(2)QDs/BiOBr heterostructures can be a promising choice for practical application of water purification.

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