详细信息
A novel synthesis of oleophylic Fe2O3/polystyrene fibers by gamma-Ray irradiation for the enhanced photocatalysis of 4-chlorophenol and 4-nitrophenol degradation ( SCI-EXPANDED收录)
文献类型:期刊文献
英文题名:A novel synthesis of oleophylic Fe2O3/polystyrene fibers by gamma-Ray irradiation for the enhanced photocatalysis of 4-chlorophenol and 4-nitrophenol degradation
作者:Wang, Ji-Chao[1,4];Li, Ying[1];Li, Heng[1];Cui, Zeng-Hui[1];Hou, Yuxia[1];Shi, Weina[2];Jiang, Kai[4];Qu, Lingbo[3];Zhang, Yu -Ping[1]
第一作者:Wang, Ji-Chao
通讯作者:Shi, WN[1];Jiang, K[2]
机构:[1]Henan Inst Sci & Technol, Coll Chem & Chem Engn, Xinxiang 453000, Henan, Peoples R China;[2]Xinxiang Univ, Coll Chem & Chem Engn, Xinxiang 453000, Henan, Peoples R China;[3]Zhengzhou Univ, Coll Chem & Mol Engn, Zhengzhou 450052, Henan, Peoples R China;[4]Henan Normal Univ, Sch Environm, Xinxiang 453000, Henan, Peoples R China
第一机构:Henan Inst Sci & Technol, Coll Chem & Chem Engn, Xinxiang 453000, Henan, Peoples R China
通讯机构:[1]corresponding author), Xinxiang Univ, Coll Chem & Chem Engn, Xinxiang 453000, Henan, Peoples R China;[2]corresponding author), Henan Normal Univ, Sch Environm, Xinxiang 453000, Henan, Peoples R China.|[110713]新乡学院化学化工学院;[11071]新乡学院;
年份:2019
卷号:379
外文期刊名:JOURNAL OF HAZARDOUS MATERIALS
收录:;WOS:【SCI-EXPANDED(收录号:WOS:000488419700028)】;
基金:This study was supported by National Natural Science Foundation of China (Nos. 51802082 and 21671059), Science and Technology Research Program of Henan Province (Nos. 182102311084 and 192102310231), Key Scientific Research Project of Colleges and Universities in Henan Province (Nos. 18A150027 and 19B150006) and Henan Postdoctoral Science Foundation.
语种:英文
外文关键词:Photocatalytic degradation; 4-chlorophenol; 4-nitrophenol; gamma-Ray; Fe2O3/PS fiber
摘要:Photocatalytic degradation by efficient and easy recyclable semiconductor-catalysts is an ideal way to solve the environmental problem. A series of Fe2O3/Polystyrene (Fe2O3/PS) composite fibers with hydrophobic property were obtained by the electrospinning and gamma-Ray irradiation methods. The gamma-Ray irradiation treatment not only formed steady micro-nano construction of nanoparticles and fiber, but also reduced the hydroxyl group on Fe2O3 surface. The high photocatalytic efficiencies of Fe2O3/PS fiber were discovered with the high content of 4-chlorophenol (4-CP) and 4-nitrophenol (4-NP), due to the synergetic effect of adsorption and degradation. The suitable adsorption capacity of Fe2O3/PS could promote the utilization of the generated hydroxyl radical(OH center dot) to directly oxidize the adsorbed pollutant molecules. Additionally, the photocatalytic activities for 4-CP and 4-NP still reached 80% and 75% in the 6th cycling and the composite fiber exhibited the good recyclability, which has the application development prospect for wastewater treatment. The mechanism of 4-CP and 4-NP decomposition was verified. Hence, the gained results could provide some insights into phenol degradation over the multifunctional and efficient catalyst.
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